Taurus Compatibility Most Least Compatible Signs MyPanditLibra passion most suitable horoscope signs are twins, aquarius, and aries. When it comes to matters of the heart, Libra seeks harmony and compatibility above all else. The Twins can bring adventure and joy to the bond, while Aquarius shares Libra's appreciation for wisdom and originality. The Ram, known for their passion, can ignite a flame in Libra's spirit. Libra and these signs create a well-rounded and fulfilling union.